I think ASP.NET MVC didn't exit at the time this question was made. It does convert anonymous objects to dictionaries internally.
Just take a look at the HtmlHelper class, for example. The method that translates objects to dictionaries is the AnonymousObjectToHtmlAttributes. It it's specifc to MVC and returns an RouteValueDictionary, however.
If you want something more generic, try this:
public static IDictionary<string,object> AnonymousObjectToDictionary(object obj)
{
    return TypeDescriptor.GetProperties(obj)
        .OfType<PropertyDescriptor>()
        .ToDictionary(
            prop => prop.Name,
            prop => prop.GetValue(obj)
        );
}
One intersting advantages of this implementation is that it returns an empty dictionary for null objects.
And here's one generic version:
public static IDictionary<string,T> AnonymousObjectToDictionary<T>(
    object obj, Func<object,T> valueSelect
)
{
    return TypeDescriptor.GetProperties(obj)
        .OfType<PropertyDescriptor>()
        .ToDictionary<PropertyDescriptor,string,T>(
            prop => prop.Name,
            prop => valueSelect(prop.GetValue(obj))
        );
}